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'Living'-chain radical polymerisation

Gennadii Vladimirovich Korolev 1
Gennadii Vladimirovich Korolev
, 
Aleksandr Petrovich Marchenko 1
Aleksandr Petrovich Marchenko
1 Institute of Problems of Chemical Physics, Russian Academy of Sciences, Chernogolovka, Moscow region
10.1070/RC2000v069n05ABEH000567
Published 30 November 1999
Communication , Volume 69, Issue 5, 409-434
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Korolev G. V., Marchenko A. P. 'Living'-chain radical polymerisation // Russian Chemical Reviews. 2000. Vol. 69. No. 5. pp. 409-434.
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Korolev G. V., Marchenko A. P. 'Living'-chain radical polymerisation // Russian Chemical Reviews. 2000. Vol. 69. No. 5. pp. 409-434.
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TY - JOUR
DO - 10.1070/RC2000v069n05ABEH000567
UR - https://rcr.colab.ws/publications/10.1070/RC2000v069n05ABEH000567
TI - 'Living'-chain radical polymerisation
T2 - Russian Chemical Reviews
AU - Korolev, Gennadii Vladimirovich
AU - Marchenko, Aleksandr Petrovich
PY - 2000
DA - 1999/11/30
PB - ANO Editorial Board of the journal Uspekhi Khimii
SP - 409-434
IS - 5
VL - 69
ER -
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@article{2000_Korolev,
author = {Gennadii Vladimirovich Korolev and Aleksandr Petrovich Marchenko},
title = {'Living'-chain radical polymerisation},
journal = {Russian Chemical Reviews},
year = {2000},
volume = {69},
publisher = {ANO Editorial Board of the journal Uspekhi Khimii},
month = {Nov},
url = {https://rcr.colab.ws/publications/10.1070/RC2000v069n05ABEH000567},
number = {5},
pages = {409--434},
doi = {10.1070/RC2000v069n05ABEH000567}
}
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Korolev, Gennadii Vladimirovich, and Aleksandr Petrovich Marchenko. “'Living'-chain radical polymerisation.” Russian Chemical Reviews, vol. 69, no. 5, Nov. 2000, pp. 409-434. https://rcr.colab.ws/publications/10.1070/RC2000v069n05ABEH000567.
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Abstract

The review is devoted to various types of compounds used as agents for 'living' radical polymerisation, such as alkoxyamines formed upon addition of the chain carrier radicals, R•, to stable nitroxyl radicals, as well as products of the addition of the radicals to transition metal complexes with different ligands, etc. In all cases, the mechanism of the action of these agents consists in their reversible dissociation A⇄R• + X•, where X• is a stable free radical or a metal-containing complex which can accept radicals R• (R• + X•→A) and thus compete with the quadratic chain termination. Particular attention is paid to the studies which allowed a quantitative formulation of the mechanism of 'living' radical polymerisation in the form of a mathematical model suitable for predicting both the parameters of the polymerisation and the properties of the resulting polymer (molecular mass and polydispersity). The bibliography includes 359 references.

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