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Mechanism of heterogeneous catalytic oxidation of organic compounds to carboxylic acids

Tamara Vital'evna Andrushkevich 1
Tamara Vital'evna Andrushkevich
, 
Yuriy Aleksandrovich Chesalov 1
Yuriy Aleksandrovich Chesalov
1 Boreskov Institute of Catalysis SB RAS, Novosibirsk
10.1070/RCR4779
Published 30 November 2017
Review , RCR4779, Volume 87, Issue 6, 586-603
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Andrushkevich T. V., Chesalov Y. A. Mechanism of heterogeneous catalytic oxidation of organic compounds to carboxylic acids // Russian Chemical Reviews. 2017. Vol. 87. No. 6. pp. 586-603.
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Andrushkevich T. V., Chesalov Y. A. Mechanism of heterogeneous catalytic oxidation of organic compounds to carboxylic acids // Russian Chemical Reviews. 2017. Vol. 87. No. 6. pp. 586-603.
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TY - JOUR
DO - 10.1070/RCR4779
UR - https://rcr.colab.ws/publications/10.1070/RCR4779
TI - Mechanism of heterogeneous catalytic oxidation of organic compounds to carboxylic acids
T2 - Russian Chemical Reviews
AU - Andrushkevich, Tamara Vital'evna
AU - Chesalov, Yuriy Aleksandrovich
PY - 2017
DA - 2017/11/30
PB - ANO Editorial Board of the journal Uspekhi Khimii
SP - 586-603
IS - 6
VL - 87
ER -
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@article{2017_Andrushkevich,
author = {Tamara Vital'evna Andrushkevich and Yuriy Aleksandrovich Chesalov},
title = {Mechanism of heterogeneous catalytic oxidation of organic compounds to carboxylic acids},
journal = {Russian Chemical Reviews},
year = {2017},
volume = {87},
publisher = {ANO Editorial Board of the journal Uspekhi Khimii},
month = {Nov},
url = {https://rcr.colab.ws/publications/10.1070/RCR4779},
number = {6},
pages = {586--603},
doi = {10.1070/RCR4779}
}
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Andrushkevich, Tamara Vital'evna, and Yuriy Aleksandrovich Chesalov. “Mechanism of heterogeneous catalytic oxidation of organic compounds to carboxylic acids.” Russian Chemical Reviews, vol. 87, no. 6, Nov. 2017, pp. 586-603. https://rcr.colab.ws/publications/10.1070/RCR4779.
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Abstract

The results of studies on the mechanism of heterogeneous catalytic oxidation of organic compounds of different chemical structure to carboxylic acids are analyzed and generalized. The concept developed by Academician G.\,K.~Boreskov, according to which the direction of the reaction is governed by the structure and bond energy of surface intermediates, was confirmed taking the title processes as examples. Quantitative criteria of the bond energies of surface compounds of oxidizable reactants, reaction products and oxygen that determine the selective course of the reaction are presented.

The bibliography includes 195 references.

Funders

Russian Academy of Sciences
0303-2016-0006

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