Home / Articles / Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior

Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior

Anna Vladimirovna Kasyanova 1, 2
Anna Vladimirovna Kasyanova
, 
Liana Raisovna Tarutina 2
Liana Raisovna Tarutina
, 
Anna Olegovna Rudenko 2
Anna Olegovna Rudenko
, 
Julia Georgievna Lyagaeva 1, 2
Julia Georgievna Lyagaeva
, 
Dmitry Andreevich Medvedev 1, 2
Dmitry Andreevich Medvedev
1 Ural Federal University named after the First President of Russia B. N. Yeltsin, Ekaterinburg
2 Institute of High-Temperature Electrochemistry, the Ural Branch of the Russian Academy of Sciences, Yekaterinburg
10.1070/RCR4928
Published 30 November 2019
Review , RCR4928, Volume 89, Issue 6, 667-692
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Kasyanova A. V. et al. Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior // Russian Chemical Reviews. 2019. Vol. 89. No. 6. pp. 667-692.
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Kasyanova A. V., Tarutina L. R., Rudenko A. O., Lyagaeva J. G., Medvedev D. A. Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior // Russian Chemical Reviews. 2019. Vol. 89. No. 6. pp. 667-692.
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TY - JOUR
DO - 10.1070/RCR4928
UR - https://rcr.colab.ws/publications/10.1070/RCR4928
TI - Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior
T2 - Russian Chemical Reviews
AU - Kasyanova, Anna Vladimirovna
AU - Tarutina, Liana Raisovna
AU - Rudenko, Anna Olegovna
AU - Lyagaeva, Julia Georgievna
AU - Medvedev, Dmitry Andreevich
PY - 2019
DA - 2019/11/30
PB - ANO Editorial Board of the journal Uspekhi Khimii
SP - 667-692
IS - 6
VL - 89
ER -
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@article{2019_Kasyanova,
author = {Anna Vladimirovna Kasyanova and Liana Raisovna Tarutina and Anna Olegovna Rudenko and Julia Georgievna Lyagaeva and Dmitry Andreevich Medvedev},
title = {Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior},
journal = {Russian Chemical Reviews},
year = {2019},
volume = {89},
publisher = {ANO Editorial Board of the journal Uspekhi Khimii},
month = {Nov},
url = {https://rcr.colab.ws/publications/10.1070/RCR4928},
number = {6},
pages = {667--692},
doi = {10.1070/RCR4928}
}
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Kasyanova, Anna Vladimirovna, et al. “Ba(Ce,Zr)O3-based electrodes for protonic ceramic electrochemical cells: towards highly compatible functionality and triple-conducting behavior.” Russian Chemical Reviews, vol. 89, no. 6, Nov. 2019, pp. 667-692. https://rcr.colab.ws/publications/10.1070/RCR4928.
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Keywords

BaCeO3
BaZrO3
electrode materials
energy conversion
proton-conducting electrolytes
Solid oxide fuel cells

Abstract

Protonic ceramic fuel cells (PCFCs) and electrolysis cells (PCECs) represent low- and intermediate-temperature electrochemical devices, which utilization allows chemical-to-electrical energy conversion with very high efficiency and low impact on the environment. To ensure long-term operability of PCFCs/PCECs as well as their up-scaling ability, a number of existing challenges, associated with chemical and thermal incompatibilities of the functional materials, should be overcome. This work aims at presenting a comprehensive overview of new electrodes materials based on barium cerate/zirconate, having structural fragments similar to that of the proton-conducting

Ba(Ce,Zr)O3 electrolytes and, correspondingly, high compatibility. Primary emphasis is paid to their functional properties such as chemical stability, thermal expansion behavior as well as transport features, which in turn determine electrochemical performance of the designed electrodes. In addition, possibility of tailoring triple-conducting materials is discussed as means of designing the electrodes with the highest electrochemical active surface area attractive for next-generation PCFCs/PCECs.

Funders

Russian Science Foundation
18-73-00001
Ministry of Education and Science of the Russian Federation
MK-1654.2019.3

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