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Supercritical fluids in chemistry

Evgenii Sergeevich Alekseev 1
Evgenii Sergeevich Alekseev
, 
Alexandr Yur'evich Alentiev 2
Alexandr Yur'evich Alentiev
, 
Anastasia Stanislavovna Belova 3
Anastasia Stanislavovna Belova
, 
Viktor Ignat'evich Bogdan 1, 4
Viktor Ignat'evich Bogdan
, 
Tatiana Veniaminovna Bogdan 1
Tatiana Veniaminovna Bogdan
, 
Aleksandra Valer'evna Bystrova 3, 5
Aleksandra Valer'evna Bystrova
, 
Elvira Rasitovna Gafarova 6
Elvira Rasitovna Gafarova
, 
Elena Nikolaevna Golubeva 1
Elena Nikolaevna Golubeva
, 
Ekaterina Andreevna Grebenik 6
Ekaterina Andreevna Grebenik
, 
Oleg Igorevich Gromov 1
Oleg Igorevich Gromov
, 
Vadim Alexandrovich Davankov 3
Vadim Alexandrovich Davankov
, 
Sergei Grigorievich Zlotin 4
Sergei Grigorievich Zlotin
, 
Mikhail Grigor'evich Kiselev 7
Mikhail Grigor'evich Kiselev
, 
Aleksei Evgenievich Koklin 4
Aleksei Evgenievich Koklin
, 
Yuriy Nikolaevich Kononevich 3
Yuriy Nikolaevich Kononevich
, 
Alexey Eduardovich Lazhko 8
Alexey Eduardovich Lazhko
, 
Valery Vasil'evich Lunin 1
Valery Vasil'evich Lunin
, 
Sergey Evgen'evich Lyubimov 3
Sergey Evgen'evich Lyubimov
,  , 
Igor Igorevich Mishanin 4
Igor Igorevich Mishanin
, 
Aziz Mansurovich Muzafarov 3, 5
Aziz Mansurovich Muzafarov
, 
Nikolay Sergeevich Nesterov 9
Nikolay Sergeevich Nesterov
, 
Alexander Yur'evich Nikolaev 3
Alexander Yur'evich Nikolaev
, 
Roman Dmitrievich Oparin 7
Roman Dmitrievich Oparin
, 
Olga Olegovna Parenago 8
Olga Olegovna Parenago
, 
Oleg Pavlovich Parenago 2
Oleg Pavlovich Parenago
, 
Yana Andreevna Pokusaeva 4
Yana Andreevna Pokusaeva
, 
Inga Alexandrovna Ronova 3
Inga Alexandrovna Ronova
, 
Anna Borisovna Solovieva 10
Anna Borisovna Solovieva
, 
Maxim Nikolaevich Temnikov 3
Maxim Nikolaevich Temnikov
, 
Petr Sergeevich Timashev 6, 10, 11
Petr Sergeevich Timashev
, 
Olga Vasil'evna Turova 4
Olga Vasil'evna Turova
, 
Evgeniya Viktorovna Filatova 4
Evgeniya Viktorovna Filatova
, 
Alexey Aleksandrovich Philippov 9
Alexey Aleksandrovich Philippov
, 
Andrey Mikhailovich Chibiryaev 9
Andrey Mikhailovich Chibiryaev
, 
1 Lomonosov Moscow State University, Faculty of Chemistry
2 A. V. Topchiev Institute of Petrochemical Synthesis, Russian Academy of Sciences, Moscow
3 A. N. Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences, Moscow
4 N.D. Zelinskii Institute of Organic Chemistry, Russian Academy of Sciences
5 N. S. Enikolopov Institute of Synthetic Polymer Materials RAS, Moscow
6 Institute for Regenerative Medicine, I. M. Sechenov First Moscow State Medical University
7 G. A. Krestov Institute of Solution Chemistry of the Russian Academy of Sciences, Ivanovo
8 Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences, Moscow
9 Boreskov Institute of Catalysis SB RAS, Novosibirsk
10 N. N. Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow
11 Federal Research Centre 'Crystallography and Photonics', Russian Academy of Sciences, Institute of Photonic Technologies, Moscow, Troitsk
10.1070/RCR4932
Published 30 November 2019
Review , RCR4932, Volume 89, Issue 12, 1337-1427
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Alekseev E. S. et al. Supercritical fluids in chemistry // Russian Chemical Reviews. 2019. Vol. 89. No. 12. pp. 1337-1427.
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Alekseev E. S., Alentiev A. Y., Belova A. S., Bogdan V. I., Bogdan T. V., Bystrova A. V., Gafarova E. R., Golubeva E. N., Grebenik E. A., Gromov O. I., Davankov V. A., Zlotin S. G., Kiselev M. G., Koklin A. E., Kononevich Y. N., Lazhko A. E., Lunin V. V., Lyubimov S. E., Mart'yanov O. N., Mishanin I. I., Muzafarov A. M., Nesterov N. S., Nikolaev A. Y., Oparin R. D., Parenago O. O., Parenago O. P., Pokusaeva Y. A., Ronova I. A., Solovieva A. B., Temnikov M. N., Timashev P. S., Turova O. V., Filatova E. V., Philippov A. A., Chibiryaev A. M., Shalygin A. S. Supercritical fluids in chemistry // Russian Chemical Reviews. 2019. Vol. 89. No. 12. pp. 1337-1427.
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TY - JOUR
DO - 10.1070/RCR4932
UR - https://rcr.colab.ws/publications/10.1070/RCR4932
TI - Supercritical fluids in chemistry
T2 - Russian Chemical Reviews
AU - Alekseev, Evgenii Sergeevich
AU - Alentiev, Alexandr Yur'evich
AU - Belova, Anastasia Stanislavovna
AU - Bogdan, Viktor Ignat'evich
AU - Bogdan, Tatiana Veniaminovna
AU - Bystrova, Aleksandra Valer'evna
AU - Gafarova, Elvira Rasitovna
AU - Golubeva, Elena Nikolaevna
AU - Grebenik, Ekaterina Andreevna
AU - Gromov, Oleg Igorevich
AU - Davankov, Vadim Alexandrovich
AU - Zlotin, Sergei Grigorievich
AU - Kiselev, Mikhail Grigor'evich
AU - Koklin, Aleksei Evgenievich
AU - Kononevich, Yuriy Nikolaevich
AU - Lazhko, Alexey Eduardovich
AU - Lunin, Valery Vasil'evich
AU - Lyubimov, Sergey Evgen'evich
AU - Mart'yanov, Oleg Nikolaevich
AU - Mishanin, Igor Igorevich
AU - Muzafarov, Aziz Mansurovich
AU - Nesterov, Nikolay Sergeevich
AU - Nikolaev, Alexander Yur'evich
AU - Oparin, Roman Dmitrievich
AU - Parenago, Olga Olegovna
AU - Parenago, Oleg Pavlovich
AU - Pokusaeva, Yana Andreevna
AU - Ronova, Inga Alexandrovna
AU - Solovieva, Anna Borisovna
AU - Temnikov, Maxim Nikolaevich
AU - Timashev, Petr Sergeevich
AU - Turova, Olga Vasil'evna
AU - Filatova, Evgeniya Viktorovna
AU - Philippov, Alexey Aleksandrovich
AU - Chibiryaev, Andrey Mikhailovich
AU - Shalygin, Anton Sergeevich
PY - 2019
DA - 2019/11/30
PB - ANO Editorial Board of the journal Uspekhi Khimii
SP - 1337-1427
IS - 12
VL - 89
ER -
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@article{2019_Alekseev,
author = {Evgenii Sergeevich Alekseev and Alexandr Yur'evich Alentiev and Anastasia Stanislavovna Belova and Viktor Ignat'evich Bogdan and Tatiana Veniaminovna Bogdan and Aleksandra Valer'evna Bystrova and Elvira Rasitovna Gafarova and Elena Nikolaevna Golubeva and Ekaterina Andreevna Grebenik and Oleg Igorevich Gromov and Vadim Alexandrovich Davankov and Sergei Grigorievich Zlotin and Mikhail Grigor'evich Kiselev and Aleksei Evgenievich Koklin and Yuriy Nikolaevich Kononevich and Alexey Eduardovich Lazhko and Valery Vasil'evich Lunin and Sergey Evgen'evich Lyubimov and Oleg Nikolaevich Mart'yanov and Igor Igorevich Mishanin and Aziz Mansurovich Muzafarov and Nikolay Sergeevich Nesterov and Alexander Yur'evich Nikolaev and Roman Dmitrievich Oparin and Olga Olegovna Parenago and Oleg Pavlovich Parenago and Yana Andreevna Pokusaeva and Inga Alexandrovna Ronova and Anna Borisovna Solovieva and Maxim Nikolaevich Temnikov and Petr Sergeevich Timashev and Olga Vasil'evna Turova and Evgeniya Viktorovna Filatova and Alexey Aleksandrovich Philippov and Andrey Mikhailovich Chibiryaev and Anton Sergeevich Shalygin},
title = {Supercritical fluids in chemistry},
journal = {Russian Chemical Reviews},
year = {2019},
volume = {89},
publisher = {ANO Editorial Board of the journal Uspekhi Khimii},
month = {Nov},
url = {https://rcr.colab.ws/publications/10.1070/RCR4932},
number = {12},
pages = {1337--1427},
doi = {10.1070/RCR4932}
}
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Alekseev, Evgenii Sergeevich, et al. “Supercritical fluids in chemistry.” Russian Chemical Reviews, vol. 89, no. 12, Nov. 2019, pp. 1337-1427. https://rcr.colab.ws/publications/10.1070/RCR4932.
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Abstract

This review analyzes the rapidly developing applications of supercritical fluids, mainly supercritical carbon dioxide, in catalysis, chemistry of high-molecular-weight compounds, and medicinal chemistry in Russia and abroad. It considers the methods of catalyst preparation based on impregnation of inorganic and organic supports with metal-containing compounds, immobilization of organometallic and metal complex reagents in matrices of oxide and polymer supports, and deposition processes employing supercritical fluids. An analysis is presented of the prospects for applying $\mathrm{CO}_2$ and some organic compounds, such as aliphatic alcohols, in sub- and supercritical states as reactants and (or) solvents for catalytic reactions of hydrocarbon isomerization and cracking, hydrogenation, dehydrogenation, oxidation, \textit{etc}., including the asymmetric reactions. The review discusses processes of synthesizing and modifying polymer materials for various purposes, including aerogels, foams, and composites impregnated with photochromes, in a supercritical fluid medium. Special attention is paid to supercritical one-pot processes, which make the techniques of obtaining new materials simpler, less expensive, and more efficient. The work investigates the effect of supercritical $\mathrm{CO}_2$ on the morphology, gas separation characteristics, and dielectric properties of polymers. One of the promising applications of supercritical fluids in medicine is the use in transplantology and pharmacology, for example, for the preparation of drug polymorphs with higher bioavailability. The review also provides an overview of the recent data on the use of EPR spectroscopy for studying the properties of supercritical fluids, including those exhibited in the vicinity of the critical point and identifying the intermediates of chemical reactions in such media.

The bibliography includes 1151 references.

Funders

Russian Foundation for Basic Research
18-29-06022
Russian Science Foundation
18-15-00401
Ministry of Education and Science of the Russian Federation
14.W03.31.0018

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