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Solid oxide fuel cells based on ceramic membranes with mixed conductivity: improving efficiency

Elena Yur'evna Pikalova 1, 2
Elena Yur'evna Pikalova
, 
Elena Grigor'evna Kalinina 1, 3
Elena Grigor'evna Kalinina
1 Ural Federal University named after the First President of Russia B. N. Yeltsin, Ekaterinburg
2 Institute of High-Temperature Electrochemistry, RAS, Ekaterinburg
3 Institute of Electrophysics, Ural Branch, Russian Academy of Sciences, Ekaterinburg
10.1070/RCR4966
Published 30 November 2020
Review , RCR4966, Volume 90, Issue 6, 703-749
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Pikalova E. Y., Kalinina E. G. Solid oxide fuel cells based on ceramic membranes with mixed conductivity: improving efficiency // Russian Chemical Reviews. 2020. Vol. 90. No. 6. pp. 703-749.
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Pikalova E. Y., Kalinina E. G. Solid oxide fuel cells based on ceramic membranes with mixed conductivity: improving efficiency // Russian Chemical Reviews. 2020. Vol. 90. No. 6. pp. 703-749.
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TY - JOUR
DO - 10.1070/RCR4966
UR - https://rcr.colab.ws/publications/10.1070/RCR4966
TI - Solid oxide fuel cells based on ceramic membranes with mixed conductivity: improving efficiency
T2 - Russian Chemical Reviews
AU - Pikalova, Elena Yur'evna
AU - Kalinina, Elena Grigor'evna
PY - 2020
DA - 2020/11/30
PB - ANO Editorial Board of the journal Uspekhi Khimii
SP - 703-749
IS - 6
VL - 90
ER -
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@article{2020_Pikalova,
author = {Elena Yur'evna Pikalova and Elena Grigor'evna Kalinina},
title = {Solid oxide fuel cells based on ceramic membranes with mixed conductivity: improving efficiency},
journal = {Russian Chemical Reviews},
year = {2020},
volume = {90},
publisher = {ANO Editorial Board of the journal Uspekhi Khimii},
month = {Nov},
url = {https://rcr.colab.ws/publications/10.1070/RCR4966},
number = {6},
pages = {703--749},
doi = {10.1070/RCR4966}
}
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Pikalova, Elena Yur'evna, and Elena Grigor'evna Kalinina. “Solid oxide fuel cells based on ceramic membranes with mixed conductivity: improving efficiency.” Russian Chemical Reviews, vol. 90, no. 6, Nov. 2020, pp. 703-749. https://rcr.colab.ws/publications/10.1070/RCR4966.
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Keywords

doped ceria
electron conductivity
grain boundary conductivity
grain conductivity
heterostructure
nanocomposite
open circuit value
oxygen ion conductivity
Solid Oxide Fuel Cell

Abstract

Modern approaches to increasing the efficiency of solid-oxide fuel cells (SOFCs) based on electrolytic membranes with mixed conductivity are considered. These approaches are based on material-science concepts (expansion of the electrolytic domain boundary due to the doping of basic oxides and development of various composite materials) and various technological solutions (application of electron-blocking layers on the anode and cathode sides, rational selection of the electrolyte thickness, and optimization of the electrolyte and electrode structures by synthesizing heterostructures). The methods of mathematical modelling of devices with an electrolytic membrane having mixed conductivity are analyzed in order to determine the most efficient design and optimal operation conditions for SOFCs. The application of nanocomposite electrolytes with a core--shell structure and salt composites is considered. Data on new design solutions --- single-layer and single-chamber SOFCs --- are presented. The prospects of the proposed approaches are evaluated. The bibliography includes 384 references.

Funders

Russian Foundation for Basic Research
20-03-00151

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